Action A1

Identification of the uncertainties related to emission factors for selected activities
This action aimed to quantify the uncertainty related to the atmospheric emission estimations for some activities that could affect the performances of air quality models, mostly in urban areas.
Expected results
– A set of PM emission factors from road dust resuspension evaluated in Barcelona and Milan, including the uncertainty quantification
– A set of NOx and primary (solid) PM emission factors from different domestic heating systems (gas, gas oil, biomass)
– A first estimation of the uncertainty related to the activity indicators of open waste burning (e.g. number and frequency of events)
– A first direct estimate of the PM wood oven pizzerias emission factor
– An estimate of NMVOC speciated emissions from solvent use sector in Milan (also including IVOC and SVOC emissions)
– An update of NMVOC chemical speciation from road transport and biomass burning (also including IVOC and SVOC emissions)
All five sub-actions and one extra covered by A1 have been concluded.
- Domestic heating systems: concluded on time. This activity followed and complemented a previous measurement campaign carried out one year before, organised by the Municipality of Milan. Main aspects and findings:
- In the context of the two measurement campaigns, more than 100 valid measurements were carried out involving different heating fuels and systems (originally planned number of valid measurements was 50, thus it represents an added value).
- The milestone for the conclusion of the domestic heating systems measurements was respected, and the D1.2 Deliverable has been transmitted on time on 31/10/2022.
- The planned output (i.e. NOx and primary PM emission factors from different domestic heating systems) has been achieved and enriched with gaseous TOC and NO2 measurements.
- This sub-activity concluded that the reference consolidated bibliography is not able to describe some recent combustion technologies, such as natural gas condensing boilers that are characterised by significantly lower NOx emissions than the conventional ones.
- Other emission sources – wood ovens: concluded on time. Emission measurements have been carried out in “real use” conditions (cooking pizzas). Main aspects and findings:
- A link with a national project (called PROFILE – PaRticOlato da FornI a LEgna funded by the Chamber of Commerce and the Italian Ministry of the Environment) was created.
- As originally planned, the measurements were mainly focussed on particulate emissions, but (as another added value) also Total Organic Carbon were measured. Thus, the obtained results are more than expected.
- The milestone for the conclusion of the wood oven measurements was respected, and the D1.3 Deliverable has been transmitted with a small delay (less than one month, within 30/11/2022) due to the unexpected difficulties in explaining some outcomes. The small delay didn’t influence the following activities of the other Actions.
- Road dust resuspension: all measurement campaigns were concluded on time both in Milan and Barcelona. More in detail:
- More activities than planned were carried out. In particular, four different methods (instead of the planned three) were used for estimating the uncertainty of the resuspension emission factors, with 11 vertical profile measurements (instead of 2 expected), 19 street porosity valid measurements (instead of 10 expected), 1 NOx dilution measurement and 8 road dust loading measurements (originally not planned) were carried out.
- As another added value for the project, the local municipal company of Milan that has in charge the ordinary street cleaning has been involved (with no charge to the project) with the goal to evaluate the influence of the street cleaning activities on the resuspension emission factor uncertainty.
- A link with the CARES – City Air Remote Emission Sensing – European Project (Horizon 2020 research and innovation programme – Grant Agreement No. 814966) was created to enrich the scientific basis of REMY about the resuspension phenomena.
- Even if the milestone for the conclusion of the resuspension measurement campaigns was respected, the D1.1 Deliverable has been transmitted late (eight months of delay by 31/07/2023) because the number of measurements, really higher compared to the planned one, took longer time for the laboratory analysis. Moreover, the experimental activities started with an initial delay due to the difficulties in obtaining the permissions for the installation of the devices in Milan. In any case, the delay in the Deliverable transmission didn’t influence the following activities of the other Actions.
- Domestic waste combustion: concluded on time except drone flights. More in detail:
- The analysis of the available scientific literature and of the results of the European Parliament Pilot Project WASTE, with the support of VITO (TA subcontractor), was done on time.
- The activity data and emission factor of domestic solid fuel burning were also used in Action A3 through receptor modelling in Krakow (Malopolska) and Raciboz (remote site in the industrial Silesia region).
- The land-base monitoring activities, involving National Associations and local citizen’s Associations, were performed on time to report the number of open burning events observed in three peri-urban areas of Milan characterised by different urban environments (construction sites, urban park and vegetable gardens, agricultural areas).
- The Local Police of Milan was involved in piloting a drone equipped with an infrared thermal camera over some test areas successfully recognizing test fires. The flights started in delay due to the unavailability of the thermal camera sensors (not in charge of the REMY project). The tests in using pilotless drones for the detection of open burning phenomena were concluded successfully.
- A new type of drone was tested. Thanks to a patented solar power technology, this drone has an autonomy of several hours and thus is able to map large areas finding automatically open-air fires. Due to the success of the activity, the City of Milan decided to acquire this type of drone for ordinary monitoring activities.
- Due to the initial difficulties in involving the drones of the Local Police of Milan and the not foreseen tests with the solar power drone, the milestone for the conclusion of drone flights activities was shifted to 30/06/2023 (10 months delay), and the D1.5 Deliverable was transmitted with a delay of 5 months by 30/06/2023. These delays didn’t influence the following activities of the other Actions.
- Other emission sources – NMVOC emissions and speciation: concluded in delay.
- The analysis of the scientific bibliography regarding the role of NMVOC – non methane volatile organic compounds – as precursors to the Secondary Organic Aerosols (SOA) was concluded on time, thus the following activities of the other Actions continued as foreseen.
- From the experimental point of view, the original plan was necessarily changed because the direct speciation of NMVOC emissions released to painting and solvent products was not feasible, having the goal to obtain representative information for this type of emission, due to the very huge number of products available. Thus, according to the aim of action A4, a measurement campaign was conducted by installing 5 canister samplers (i.e. air samplers capable of filling an initially evacuated canister by action of the flow-controlled pump) in different areas of Milan. It was the unique solution able to combine the goals of the campaign, the logistic constraints and the time scheduling. The canisters collected atmospheric air for 7 days (differentiating working days and weekdays), and the samples were characterised in the laboratory (UNI EN ISO 16017) to measure the concentration of some NMVOC species that the bibliography (see above) indicated as more interesting for the REMY goals.
- as a consequence of the encountered difficulties for the experimental activities, the milestone for the NMVOC speciation was shifted to 31/07/2023 (ten months of delay), and the D1.4 Deliverable has been transmitted with a delay of nine months (31/07/2023).
- Other emission sources – cooking activities: new activity, originally not planned. The conclusion of the sub-activity “wood ovens” suggested to more investigate the particulate and gaseous emissions from cooking activities. In fact, according to the obtained results of the “wood ovens” activities and the few available scientific bibliography (mainly American and Asian), the particulate and gaseous emissions from some techniques of cooking preparation (i.e. grilled, fried…) could be an important aspect to take into account, according to the goals of the REMY project.
- An experimental activity was conducted to estimate the emission factor of TOC and TPS through different cooking methods like frying, grilling and stewing of different foods. The activities were carried out in an accredited laboratory using the same techniques adopted for the wood ovens in order to have comparable results.
- Moreover, thanks to the Research Council for Agriculture and Environment of the Italian Ministry for Agricultural and Food, food habits regarding food consumption and cooking methods in Northern Italy were retrieved, and the corresponding annual emissions were estimated.
- The experimental activities and the final Deliverable were concluded before the end of the REMY project. It represents a totally added value compared to the planned results.